Suggestions by @williamvisnosky

Edward Norton

as Daredevil in Spider-Man (1999)

Score: +1

Henry Rollins

as The Punisher in Spider-Man (1999)

Score: +4

Ryan Phillippe

as Hobgoblin in Spider-Man (1999)

Score: +1

John Malkovich

as Vulture in Spider-Man (1999)

Score: +1

Mark Hamill

as Green Goblin in Spider-Man (1999)

Score: +1

Claire Danes

as Mary Jane Watson in Spider-Man (1999)

Score: +1

Macaulay Culkin

as Spider-Man in Spider-Man (1999)

Score: +1

Christopher Lloyd

as Uncle Ben in Spider-Man (1999)

Score: +1

Maggie Smith

as Aunt May in Spider-Man (1999)

Score: +1

Tommy Lee Jones

as Senator Robert Kelly in X-Men (1996)

Score: +1

Tim Curry

as Mister Sinister in X-Men (1996)

Score: +1

Michelle Pfeiffer

as Emma Frost in X-Men (1996)

Score: +1

Angelina Jolie

as Psylocke in X-Men (1996)

Score: +1

Alicia Silverstone

as Scarlett Witch in X-Men (1996)

Score: +1

Jonathan Brandis

as Quicksilver in X-Men (1996)

Score: +1

Donald Sutherland

as Magneto in X-Men (1996)

Score: +1

Sharon Stone

as Mystique in X-Men (1996)

Score: +1

Ron Perlman

as Juggernaut in X-Men (1996)

Score: +1

Dolph Lundgren

as Sabretooth in X-Men (1996)

Score: +2

Matthew Lillard

as Pyro in X-Men (1996)

Score: +1