Suggestions by @harrissyed

The Jigsaw Killer

as Saw's Villain in Good VS Evil

Score: +1

Satan Himself

as The Bible's Villain in Good VS Evil

Score: +1

Griffith (Berserk)

as Berserk's Villain in Good VS Evil

Score: +3

Zeus (God of War)

as Kratos' Villain in Good VS Evil

Score: +1

Mr. Burns

as The Simpsons' Villain in Good VS Evil

Score: +1

Queen Beryl

as Sailor Moon's Villain in Good VS Evil

Score: +3

Lord Frieza

as Dragon Ball's Villain in Good VS Evil

Score: +2

Omni Consumer Products

as RoboCop's Villain in Good VS Evil

Score: +1

Ingsoc

as 1984's Villain in Good VS Evil

Score: +1

Templar Order

as Assassin's Creed Villain in Good VS Evil

Score: +1

Republic of Gilead

as The Handmaid's Tale Villain in Good VS Evil

Score: +1

Vought

as The Boys' Villain in Good VS Evil

Score: +1

Homelander

as The Boys' Villain in Good VS Evil

Score: 0

Thragg

as Invincible's Villain in Good VS Evil

Score: +3

Darkseid

as Justice League's Villain in Good VS Evil

Score: +1

Doctor Doom

as Fantastic Four's Villain in Good VS Evil

Score: +1

Thanos

as Avengers' Villain in Good VS Evil

Score: +1

Magneto (Erik Lehnsherr)

as X-Men's Villain in Good VS Evil

Score: +3

Tetsuo Shima

as AKIRA's Villain in Good VS Evil

Score: +1

Skynet

as Terminator's Villain in Good VS Evil

Score: +3